Effect of side‐chain length on the electrospinning of perfluorosulfonic acid ionomers

Published in Journal of Polymer Science Part A: Polymer Chemistry, vol. 51(1), pp. 118–128 (2013) · first published 11 September 2012
DOI: 10.1002/pola.26286

Summary

Perfluorosulfonic acid (PFSA) ionomers such as Nafion (long side chain) and Aquivion (short side chain) are the benchmark proton-exchange membrane materials for fuel cells, and turning them into nanofibres by electrospinning is a promising route to better-structured membranes. However, pure ionomers electrospin poorly because they lack the chain entanglement needed to form a stable jet, so a carrier polymer is usually required. This study examines how the length of the ionomer side chain influences electrospinning behaviour, comparing long- and short-side-chain PFSA and the morphology of the fibres they form. The findings help define the processing conditions for producing PFSA nanofibre mats aimed at fuel-cell membrane applications.

Authors & Affiliations

Topics

Fuel Cell Membranes Proton-Exchange Membranes Ionomers Energy Materials

Materials

Perfluorosulfonic Acid (PFSA) Nafion

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