A Green Method for Bacterial Cellulose Electrospinning Using 1-Butyl-3-Methylimidazolium Acetate

Published in Polymers, vol. 17(9), 1162 (2025) · MDPI · Open access, CC BY
DOI: 10.3390/polym17091162

Summary

Bacterial cellulose is exceptionally pure and highly crystalline, but the same hydrogen bonding and high molecular weight that give it those qualities make it impossible to melt and very hard to dissolve, so processing it usually means resorting to aggressive and toxic solvents. This study demonstrates a greener route to electrospun bacterial cellulose fibres by screening ionic liquids as solvents - 1-butyl-3-methylimidazolium acetate alongside two imidazolium alternatives - and identifying conditions under which the material can be spun successfully. The approach removes the most objectionable chemistry from the process and opens bacterial cellulose to fibre applications that its solubility had previously ruled out.

Authors & Affiliations

  • Erlantz Vasili
    Department of Civil and Industrial Engineering, University of Pisa, Italy
  • Bahareh Azimi Corresponding
    Department of Civil and Industrial Engineering, University of Pisa, Italy
  • Mahendra P. Raut
    School of Chemical, Materials and Biological Engineering, University of Sheffield, UK
  • David A. Gregory
    School of Chemical, Materials and Biological Engineering, University of Sheffield, UK
  • Antonio Mele
    School of Chemical, Materials and Biological Engineering, University of Sheffield, UK
  • Bing Liu
    School of Chemical, Materials and Biological Engineering, University of Sheffield, UK
  • Kai Römhild
    Thuringian Institute for Textile and Plastics Research (TITK), Rudolstadt, Germany
  • Marcus Krieg
    Thuringian Institute for Textile and Plastics Research (TITK), Rudolstadt, Germany
  • Frederik Claeyssens
    School of Chemical, Materials and Biological Engineering, University of Sheffield, UK
  • Patrizia Cinelli
    Department of Civil and Industrial Engineering, University of Pisa, Italy

Linari Electrospinning Systems

Electrospinning bench apparatus with rotating collector
The solutions were spun on an electrospinning bench apparatus (Linari Engineering S.r.l., Pisa, Italy) equipped with a rotating collector and a static coagulation bath - a configuration combining the Easy Drum rotary unit with the HVG-CONT-LCD high voltage control unit of the Starter Kit.

Topics

Green Electrospinning Cellulose Dissolution Sustainable Materials Wet Spinning Bath

Materials

Bacterial cellulose Imidazolium ionic liquids
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